Photo-controlled degradation of natural rubber (Record no. 64903)

MARC details
000 -LEADER
fixed length control field 01588nam a2200181Ia 4500
100 ## - MAIN ENTRY--AUTHOR NAME
Personal name Solanky S S
245 #0 - TITLE STATEMENT
Title Photo-controlled degradation of natural rubber
260 ## - PUBLICATION, DISTRIBUTION, ETC. (IMPRINT)
Name of publisher Journal of Rubber Research
Year of publication 2000
300 ## - PHYSICAL DESCRIPTION
Number of Pages 76-94
520 ## - SUMMARY, ETC.
Summary, etc The chain cleavage mechanisms during hydrogen peroxide catalysed photo-oxidative degradation of high molecular weight natural rubber, which was described as producing liquid natural rubber is elucidated. NR is photolysed in toluene solution(2.5 wt.;) in a photoreactor at 30 oC under atmospheric air and nitrogen, separately, with a 400 W medium pressure mercury vapour lamp( =>_290nm) with constant stirring in the presence of hydrogen peroxide and/or titanium dioxide. The decrease in viscosity-average molecular weight(Mv) was determined by viscosity measurements. The photoproducts were characterised by FT-IR, 1H and 13C NMR spectroscopies. Burfields and the present results gave indication for chain cleavages resulting from the classical free-radical oxidation process rather than a direct reaction of hydroxy radical at the methylene-methylene bond. The hydrogen peroxide and/or allylic hydroperoxides acts as photoinitiator by producing hydroxy radicals and/or alkoxy radicals. Moreover, the concomitant addition of 1 O2 (singlet oxygen) via the well known ene reaction producing hydroperoxides, can not be neglected.
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Photo-controlled oxidation
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Rubber degradation
700 ## - ADDED ENTRY--PERSONAL NAME
Personal name Campistron I
700 ## - ADDED ENTRY--PERSONAL NAME
Personal name Reyx D
700 ## - ADDED ENTRY--PERSONAL NAME
Personal name Singh R P
942 ## - ADDED ENTRY ELEMENTS (KOHA)
Koha item type Journals
Holdings
Withdrawn status Lost status Damaged status Not for loan Home library Current library Shelving location Date acquired Serial Enumeration / chronology Koha item type
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