In situ epoxidization of natural rubber latex by performic acid and the kinetics of the reaction (Record no. 60930)

MARC details
000 -LEADER
fixed length control field 01598nam a2200205Ia 4500
100 ## - MAIN ENTRY--AUTHOR NAME
Personal name George B
245 #0 - TITLE STATEMENT
Title In situ epoxidization of natural rubber latex by performic acid and the kinetics of the reaction
260 ## - PUBLICATION, DISTRIBUTION, ETC. (IMPRINT)
Name of publisher Indian Journal of Natural Rubber Research
Year of publication 1992
300 ## - PHYSICAL DESCRIPTION
Number of Pages 179-187
520 ## - SUMMARY, ETC.
Summary, etc Epoxidation of natural rubber latex stabilised with a nonionic surfactant was carried out with performica acid generated in situ. The reaction was performed at 30, 45, 50 and 60 degree C at a dry rubber content (DRC) of 20 and concentration of formic acid and hydrogen peroxide 0.955 and 3.75 modle dm3 respectively in the aqueous phase of the latex. Product characterization by 1H NMR and IR spectroscopic methods indicated significant influence of temperature on the extent of epoxidation as well as ring opening reactions. Epoxidation to the extent of 25-35 mole per cent could be reached without ring opening. The concentration of ring opened products at higher levels of epoxidation was found to be low. The reaction followed pseudo-first order kinetics with the formation of performic acid as the rate dtermining step. This was further confirmed by carrying out the reaction at 10 and 15 per cent DRC keeping the formic acid and hydrogen peroxide concentrations in the aqueous phase the same.
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Epoxidization
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Epoxidization kinetics
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Natural rubber latex
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Performic acid
650 ## - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical Term Ring opening reactions
700 ## - ADDED ENTRY--PERSONAL NAME
Personal name Abraham S
700 ## - ADDED ENTRY--PERSONAL NAME
Personal name Mathew N M
942 ## - ADDED ENTRY ELEMENTS (KOHA)
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